Should we send some type of formal contract ending and request something back?
If it was me I'd just delete the images to the extent possible (I know some of the sites only allow you to delete a certain percentage at one time, and Dreamstime has that 3 month rule).
To my knowledge there is nothing you have to send or request to delete your portfolio on any of the microstock sites, with the except of the sites that have retention policies as mentioned above. I have no idea why you would send a contract to end a relationship. You already agreed to contractual terms when you signed up and submitted the photos.